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| Open AccessExtreme magnetoresistance at high-mobility oxide heterointerfaces with dynamic defect tunability
Extreme magnetoresistance is characterized by a large and non-saturating magnetoresistance. Typically, it is observed in materials with compensated bandstructures, however, here, Christensen et al demonstrate a large and non-saturating magnetoresistance in a γAl2O3/SrTiO3 heterostructure, which is related to disorder, rather than the materials bandstructure.
- D. V. Christensen
- , T. S. Steegemans
- & N. Pryds
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Article
| Open AccessStrong microwave squeezing above 1 Tesla and 1 Kelvin
At the quantum limit, vacuum fluctuations determine the precision with which a signal can be measured. In this work the authors use a technique known as squeezing to greatly reduce the vacuum fluctuation noise present at microwave frequencies.
- Arjen Vaartjes
- , Anders Kringhøj
- & Jarryd J. Pla
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Article
| Open AccessEvidence for multiferroicity in single-layer CuCrSe2
The authors observe multiferroicity in a single-layer non van der Waals material, CuCrSe2. The coexistence of room-temperature ferroelectricity and ferromagnetism up to 120 K is corroborated by a set of comprehensive experimental techniques.
- Zhenyu Sun
- , Yueqi Su
- & Baojie Feng
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Article
| Open AccessHigh spin axion insulator
Existing proposals of axion insulators are limited to spin-1/2 systems. Here the authors put forward a concept of a high spin axion insulator with several peculiar properties, such as the absence of gapless surface states and tunability of the axion field by an external magnetic field.
- Shuai Li
- , Ming Gong
- & X. C. Xie
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Article
| Open AccessCentimeter-scale nanomechanical resonators with low dissipation
Exploring new mechanics regime, researchers created centimeter-long, nanometer-thin resonators, achieving unmatched room temperature mechanical isolation via cutting edge nanoengineering and machine learning design; rivaling cryogenic counterparts.
- Andrea Cupertino
- , Dongil Shin
- & Richard A. Norte
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Article
| Open AccessTime-resolved THz Stark spectroscopy of molecules in solution
Stark spectroscopy of molecules in liquid solutions was once challenging due to orientation effects, solved by freezing but limiting ambient studies. Now, THz Stark spectroscopy with intense terahertz pulses enables dynamic analysis of molecules in both non-polar and polar solvents at any temperature, advancing conventional methods.
- Bong Joo Kang
- , Egmont J. Rohwer
- & Thomas Feurer
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Article
| Open AccessUniversal scaling in real dimension
Universality of critical behaviour of O(N) field theories on regular homogeneous lattices is established, but open questions remain for more complex lattices. Bighin et al. study universality on a non-homogeneous graph showing that its scaling theory is controlled by a single parameter, the spectral dimension.
- Giacomo Bighin
- , Tilman Enss
- & Nicolò Defenu
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Article
| Open AccessReduction of precious metal ions in aqueous solutions by contact-electro-catalysis
Currently, precious metal recovery from e-waste water is usually performed by liquid extraction or sorbent processes. Here, the authors show the untapped potential of dielectric insulators as catalysts for the 1-step selective recovery of gold in aqueous solutions by contact-electrocatalysis.
- Yusen Su
- , Andy Berbille
- & Zhong Lin Wang
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Article
| Open AccessEfficient multimode Wigner tomography
Standard ways of characterising quantum states incur exponential overhead. Here, the authors consider the task of reconstructing density matrices of multimode continuous variable systems, and demonstrate a method which scales polynomially with the system size, provided the state lies in a polynomial dimensional subspace.
- Kevin He
- , Ming Yuan
- & David I. Schuster
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Article
| Open AccessSqueezed light from an oscillator measured at the rate of oscillation
The authors demonstrated an unprecedented level of polarization squeezing of light generated by an atomic ensemble, and a new regime of continuous quantum measurements on a macroscopic material oscillator.
- Christian Bærentsen
- , Sergey A. Fedorov
- & Eugene S. Polzik
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Article
| Open AccessDeterministic positioning and alignment of a single-molecule exciton in plasmonic nanodimer for strong coupling
Realising single molecule strong coupling with plasmons achieving both deterministic molecule positioning and dipole alignment with the mode field has proven challenging so far. Here, the authors fill this gap by placing a single molecular emitter in the gap centre of an Au nanodimer system.
- Renming Liu
- , Ming Geng
- & Lin Wu
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Article
| Open AccessCrossover from gas-like to liquid-like molecular diffusion in a simple supercritical fluid
Within the phase diagram of pure substances, the supercritical state is not fully understood. Here the authors experimentally observe a gas-like to liquid-like crossover in the self-dynamics of supercritical fluid methane upon pressure increase.
- Umbertoluca Ranieri
- , Ferdinando Formisano
- & Livia E. Bove
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Article
| Open AccessInverted device architecture for high efficiency single-layer organic light-emitting diodes with imbalanced charge transport
Efficient organic light-emitting diodes require a multilayer architecture to confine charge recombination to the emissive layer. Here, authors demonstrate efficient single-layer devices for emitters with imbalanced charge transport without the need of additional charge transport or blocking layers.
- Xiao Tan
- , Dehai Dou
- & Gert-Jan A. H. Wetzelaer
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Article
| Open AccessSpin-orbit torque manipulation of sub-terahertz magnons in antiferromagnetic α-Fe2O3
Antiferromagnetic spintronics offer high speed operations, and reduced issues with stray fields compared to ferromagnetic systems, however, antiferromagnets are typically more challenging to manipulate electrically. Here, Yang, Kim, and coauthors demonstrate electrical control of magnon dispersion and frequency in an α-Fe2O3/Pt heterostructure.
- Dongsheng Yang
- , Taeheon Kim
- & Hyunsoo Yang
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Article
| Open AccessUltrastrong magnon-magnon coupling and chiral spin-texture control in a dipolar 3D multilayered artificial spin-vortex ice
Extending magnetic nanostructures into three dimensions offers a vast increase in potential functionalities, but this typically comes at the expense of ease of fabrication and measurement. Here, Dion et al. demonstrate an approach to creating three dimensional magnetic nanostructures while retaining easy fabrication and readout of established two dimensional approaches.
- Troy Dion
- , Kilian D. Stenning
- & Jack C. Gartside
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Article
| Open AccessTracking nuclear motion in single-molecule magnets using femtosecond X-ray absorption spectroscopy
The authors use femtosecond K-edge X-ray absorption spectroscopy to follow nuclear motion in a manganese-based tri-nuclear single-molecule magnet, and resolve changes in bond lengths on the order of hundreds of ångströms and on sub-picosecond timescales.
- Kyle Barlow
- , Ryan Phelps
- & J. Olof Johansson
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Article
| Open AccessDynamics of growing carbon nanotube interfaces probed by machine learning-enabled molecular simulations
There is a lack of atomic level insight on the role of defects on carbon nanotubes' growth. Here, authors present a machine learning force field to drive near-microsecond simulations the entire growth process of this material, unveiling mechanisms of defect formation and healing.
- Daniel Hedman
- , Ben McLean
- & Feng Ding
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Article
| Open AccessOptical vectorial-mode parity Hall effect: a case study with cylindrical vector beams
This study uses a customized metasurface to unveil a distinct parity Hall effect in degenerate optical vectorial modes. This work realizes the advances in meta-devices and showcases new possibilities for manipulating optical fields based on parity.
- Changyu Zhou
- , Weili Liang
- & Xiaocong Yuan
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Article
| Open AccessPlasma electron acceleration driven by a long-wave-infrared laser
The laser pulses that drive most laser wakefield accelerators have wavelengths near 1 micrometer and peak power > 100 terawatts. Here, the authors drive plasma wakes with 10 micrometer, 2-terawatt pulses, yielding relativistic electron beams with a collimated, narrow-energy-bandwidth component.
- R. Zgadzaj
- , J. Welch
- & M. C. Downer
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Article
| Open AccessCoherent electric field control of orbital state of a neutral nitrogen-vacancy center
Color centers in diamond have been proposed as a link between remote superconducting units in hybrid quantum systems, where their orbital degree of freedom is utilized. Here the authors report coherent electric-field control of the orbital state of a neutral NV center in diamond.
- Hodaka Kurokawa
- , Keidai Wakamatsu
- & Hideo Kosaka
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Article
| Open AccessA multifunctional smart field-programmable radio frequency surface
A field-programmable radio frequency surface (FPRFS) is proposed that can implement arbitrary antennas and impedance matching networks. An asymmetric excitation scheme is demonstrated to ensure radiation efficiency independent of the number of FPRFS switches.
- Tianzhi Li
- , Yang Yu
- & Efstratios Skafidas
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Article
| Open AccessHighest fusion performance without harmful edge energy bursts in tokamak
Damaging energy bursts in a tokamak are a major obstacle to achieving stable high-fusion performance. Here, the authors demonstrate the use of adaptive and machine-learning control to optimize the 3D magnetic field to prevent edge bursts and maximize fusion performance in two different fusion devices, DIII-D and KSTAR.
- S. K. Kim
- , R. Shousha
- & E. Kolemen
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Article
| Open AccessCavity-enhanced photon indistinguishability at room temperature and telecom wavelengths
Carbon nanotube-based single photon emitters allow for room-temperature operation, but suffer from vanishing indistinguishability due to strong dephasing. Following a theoretical proposal, the authors tackle the problem experimentally by using a cavity to enhance the photon coherence time and the emission spectral density in the regime of incoherent good cavity-coupling.
- Lukas Husel
- , Julian Trapp
- & Alexander Högele
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Article
| Open AccessHigh-temperature concomitant metal-insulator and spin-reorientation transitions in a compressed nodal-line ferrimagnet Mn3Si2Te6
The coupling between topological electronic properties and magnetic order offers a promising route for magnetoelectric control with great potential for both applications and fundamental physics. Here, Susilo et al demonstrate the rich tunability of magnetic properties in nodal-line magnetic semiconductor Mn3Si2Te6 using pressure as control knob.
- Resta A. Susilo
- , Chang Il Kwon
- & Jun Sung Kim
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Article
| Open AccessUnconventional magnetism mediated by spin-phonon-photon coupling
Here Pantazopoulos, Feist, García-Vidal, and Kamra explore the combination spin, phonon and photon coupling in a system of magnetic nanoparticles, and find that it leads to an emergent spin-spin interaction. This interaction is long-range and leads to an unconventional form of magnetism that can exhibit strong magnetization at temperatures very close to the critical temperature.
- Petros Andreas Pantazopoulos
- , Johannes Feist
- & Akashdeep Kamra
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Article
| Open AccessUnconventional superconductivity without doping in infinite-layer nickelates under pressure
The authors theoretically study the pressure dependence of the phase diagram of the nickelate PrNiO2 with and without Sr doping. At high pressure, they find that the superconducting dome is significantly enhanced in both Tc and doping-range of superconductivity compared with ambient pressure, with a maximal Tc of 100 K around 100 GPa in absence of external doping.
- Simone Di Cataldo
- , Paul Worm
- & Karsten Held
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Article
| Open AccessMechanically induced correlated errors on superconducting qubits with relaxation times exceeding 0.4 ms
Significant efforts have been dedicated to understanding the mechanisms of decoherence in superconducting qubits. Here, using time-resolved error measurements, the authors link errors present in transmon qubits based on Nb electrodes to mechanical vibrations of a commonly used pulse tube cooler.
- Shingo Kono
- , Jiahe Pan
- & Tobias J. Kippenberg
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Article
| Open AccessEfficient characterizations of multiphoton states with an ultra-thin optical device
Shadow tomography is efficient for quantum state characterization. Here, the authors implement shadow tomography on photonic states with a single metasurface, which alleviates the complexity in measurement
- Kui An
- , Zilei Liu
- & He Lu
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Article
| Open AccessPolar Bloch points in strained ferroelectric films
Authors predict polar Bloch points with negative capacitance in tensile-strained ultrathin ferroelectric PbTiO3 film by phase-field simulations, observing their polarization structures by scanning transmission electron microscopic imaging.
- Yu-Jia Wang
- , Yan-Peng Feng
- & Xiu-Liang Ma
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Article
| Open AccessSpin-orbit-splitting-driven nonlinear Hall effect in NbIrTe4
Previous work proposed the Berry curvature dipole as the mechanism of the nonlinear Hall effect. Lee et al. establish the sign-changing Berry curvature hot spots from spin-orbit split bands as the origin of the Berry curvature dipole and link it to the nonlinear Hall effect in the topological semimetal NbIrTe4.
- Ji-Eun Lee
- , Aifeng Wang
- & Hyejin Ryu
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Article
| Open AccessFrequency comb generation via synchronous pumped χ(3) resonator on thin-film lithium niobate
Here the authors use on-chip amplitude and phase modulation to synchronously pump a resonator on thin-film lithium niobate for frequency comb generation. They find that pulsed pumping significantly mitigates stimulated Raman scattering and improves the overall efficiency of the device.
- Rebecca Cheng
- , Mengjie Yu
- & Marko Lončar
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Matters Arising
| Open AccessTechnical challenges of studying the impact of plasma components on the efficacy of lipid nanoparticles for vaccine and therapeutic applications
- Jens B. Simonsen
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Article
| Open AccessLarge transverse thermoelectric effect induced by the mixed-dimensionality of Fermi surfaces
The conversion between longitudinal heat flow and transverse charge current is a promising energy harvesting technology. Here, the authors show the large transverse thermoelectric effect induced by the mixed-dimensionality of Fermi surfaces.
- Hikari Manako
- , Shoya Ohsumi
- & D. Aoki
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Article
| Open AccessPhase-separated droplets swim to their dissolution
Here the authors identify a generic coupling in phase-separated liquids between motility and phase equilibria perturbations: phase-separated droplets swim to their dissolution. This suggests alternative transport mechanism for biomolecular condensates.
- Etienne Jambon-Puillet
- , Andrea Testa
- & Eric R. Dufresne
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Article
| Open AccessLevitation and dynamics of bodies in supersaturated fluids
When a solid object is placed in a supersaturated environment, it can exhibit interesting dynamics. Spagnolie et al. conducted an experiment using raisins and 3D-printed bodies in carbonated water and found that the motion of the solid object is influenced by the accumulation and release of bubbles as they reach the surface.
- Saverio E. Spagnolie
- , Samuel Christianson
- & Carsen Grote
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Article
| Open AccessNeutron scattering and neural-network quantum molecular dynamics investigation of the vibrations of ammonia along the solid-to-liquid transition
Through neutron scattering experiments coupled with machine learning, the authors uncover the strong role of nuclear quantum effects in the dynamics of ammonia in both its solid and technologically relevant liquid phase.
- T. M. Linker
- , A. Krishnamoorthy
- & P. D. Vashishta
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Article
| Open AccessA linear response framework for quantum simulation of bosonic and fermionic correlation functions
As quantum simulations advance, the ability to measure response functions of simulated systems becomes increasingly important. Here the authors present a linear response framework for computing fermionic and bosonic response functions on a quantum computer, demonstrating advantages over existing methods.
- Efekan Kökcü
- , Heba A. Labib
- & A. F. Kemper
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Article
| Open AccessRevealing the three-dimensional arrangement of polar topology in nanoparticles
Low-dimensional ferroelectric systems are predicted to have topologically nontrivial polar structures, such as vortices or skyrmions. Here authors present atomic-scale 3D topological polar structures in BaTiO3 nanoparticles using atomic electron tomography and revealed their size-dependent transitions.
- Chaehwa Jeong
- , Juhyeok Lee
- & Yongsoo Yang
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Article
| Open AccessObservation of interlayer plasmon polaron in graphene/WS2 heterostructures
Here, the authors report the observation of an interlayer plasmon polaron in heterostructures composed of graphene and monolayer WS2. This is manifested in the ARPES spectra as a strong quasiparticle peak accompanied by several carrier density-dependent shake-off replicas around the WS2 conduction band minimum.
- Søren Ulstrup
- , Yann in ’t Veld
- & Jyoti Katoch
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Article
| Open AccessVisualizing the gas-sensitive structure of the CuZn surface in methanol synthesis catalysis
Industrial methanol synthesis uses materials based on Cu and ZnO. We present high-resolution imaging of active surfaces which reveals how Zn species are transported at the active Cu interface in diffusion processes controlled by the reactant gas composition.
- Sigmund Jensen
- , Mathias H. R. Mammen
- & Jeppe V. Lauritsen
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Article
| Open AccessControlling chaos using edge computing hardware
Creating accurate digital twins and controlling nonlinear systems displaying chaotic dynamics is challenging due to high system sensitivity to initial conditions and perturbations. The authors introduce a nonlinear controller for chaotic systems, based on next-generation reservoir computing, with improved accuracy, energy cost, and suitable for implementation with field-programmable gate arrays.
- Robert M. Kent
- , Wendson A. S. Barbosa
- & Daniel J. Gauthier
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Article
| Open AccessSpontaneous persistent activity and inactivity in vivo reveals differential cortico-entorhinal functional connectivity
Cortico-entorhinal interactions remain poorly understood. Here, the authors demonstrate that a model of interacting networks predicts spontaneous persistent activity and inactivity in the medial, but not lateral, entorhinal cortex in vivo.
- Krishna Choudhary
- , Sven Berberich
- & Mayank R. Mehta
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Article
| Open AccessSemantic regularization of electromagnetic inverse problems
Solving ill-posed inverse problems require regularisation based on prior knowledge, which is formulated mathematically or learned from data. Here, the authors demonstrated the concept of semantic regularisation based on large language model to circumvent the current limitation.
- Hongrui Zhang
- , Yanjin Chen
- & Lianlin Li
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Article
| Open AccessProbing the activated complex of the F + NH3 reaction via a dipole-bound state
Experimental characterization of the transition state in chemical reactions is challenging due to its transient nature. Here, Zhang et al. observe quantum states near the activated complex region of the F + NH3 → HF + NH2 reaction via a dipole-bound state of the FNH3- anion formed upon photodetachment, which allows probing regions of reactive potential energy surfaces out of the Franck-Condon-active areas.
- Rui Zhang
- , Shuaiting Yan
- & Chuangang Ning
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Article
| Open AccessFree-standing ultrathin silicon wafers and solar cells through edges reinforcement
Lightweight and flexible thin crystalline silicon solar cells have huge market potential but remain relatively unexplored. Here, authors present a thin silicon structure with reinforced ring to prepare free-standing 4.7-μm 4-inch silicon wafers, achieving efficiency of 20.33% for 28-μm solar cells.
- Taojian Wu
- , Zhaolang Liu
- & Wenzhong Shen
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Article
| Open AccessQuantum fluctuations lead to glassy electron dynamics in the good metal regime of electron doped KTaO3
An electron glass state usually occurs in disordered insulating systems. Here the authors report evidence of glassy dynamics of conduction electrons in an electron-doped quantum paraelectric material KTaO3, in the good metal regime, where quantum fluctuations play an important role.
- Shashank Kumar Ojha
- , Sankalpa Hazra
- & Srimanta Middey
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Article
| Open AccessTopologically trivial gap-filling in superconducting Fe(Se,Te) by one-dimensional defects
Previous measurements of FeSe0.45Te0.55 found one-dimensional (1D) defects that were interpretated as domain walls hosting propagating Majorana topological modes. Here, the authors reveal that these 1D defects correspond to sub-surface debris and show that the filling of the superconducting gap on these defects is topologically trivial.
- A. Mesaros
- , G. D. Gu
- & F. Massee
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Article
| Open AccessRevealing the spatial nature of sublattice symmetry
Sublattice symmetry has long been synonymous with chiral symmetry when it comes to topological classification. Here, the authors challenge this notion by systematically investigating sublattice symmetry and revealing its spatial nature with a precise description in terms of symmetry algebra and representation.
- Rong Xiao
- & Y. X. Zhao
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Article
| Open AccessSymmetry breaking in optimal transport networks
Finding an optimal shape for transport networks, represented as multilayer structures, is a challenging problem. The authors propose analytical and computational frameworks to analyze sharp transitions from symmetric to asymmetric shapes in optimal networks, that can be applied for planning and development of improved multimodal transportation systems within a city.
- Siddharth Patwardhan
- , Marc Barthelemy
- & Filippo Radicchi
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