Materials science articles within Nature Communications

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  • Article
    | Open Access

    Copolymers prepared by controlled radical chain-growth polymerizations usually contain ill-defined monomer sequences. Here, successive feeds of donor and acceptor comonomers are used to control the primary structure of the synthesized copolymers with very high accuracy.

    • Mirela Zamfir
    •  & Jean-François Lutz

  • Article |

    Light-emitting diodes are attractive sources of light used in an increasing range of applications. This study presents a novel europium-based phosphor that gives rise to a substantial reduction in the glare that often makes LEDs uncomfortable to the human eye.

    • Hisayoshi Daicho
    • , Takeshi Iwasaki
    •  & Hideo Hosono

  • Article |

    Nanoporous zeotypes have applications as catalysts and in gas separation, but they are usually produced as moderately dense silicates and aluminosilicates with relatively low capacities for gas uptake. Here, zeotype structures are reported with very low densities and high total specific pore volumes.

    • Benjamin T.R. Littlefield
    •  & Mark T. Weller

  • Article |

    The degree of polydispersity of colloidal suspensions is known to have consequences for their physical properties. Kuritaet al. present a general method for determining the sizes of individual particles, and thus the polydispersity, using only the coordinates of the centre positions of spherical particles.

    • Rei Kurita
    • , David B. Ruffner
    •  & Eric R. Weeks

  • Article |

    Strain in Si nanostructures is used to achieve higher carrier mobility, making these devices candidates for the next generation of transistors. Minamisawaet al. fabricate silicon nanowires subject to elastic tensile strain up to 4.5%, exceeding the limit achievable with the use of SiGe virtual substrates.

    • R.A. Minamisawa
    • , M.J. Süess
    •  & H. Sigg

  • Article |

    T- and X-shaped polyphilic liquid crystals can generate ordered structures with potential nanotechnology applications. Here, the inability of polyphiles to achieve optimal packing and complete nanophase separation is exploited to produce a flexible two-dimensional honeycomb with giant octagonal and square cylinders.

    • Feng Liu
    • , Robert Kieffer
    •  & Carsten Tschierske

  • Article
    | Open Access

    The physical properties of organic metals have generally been described in terms of a highly correlated Luttinger liquid. Using angle-resolved photoelectron spectroscopy, Kisset al. measure the Fermi surface of (BEDT-TTF)3Br(pBIB), and find that, in contrast to other systems, it can be described as a Fermi liquid.

    • T. Kiss
    • , A. Chainani
    •  & S. Shin

  • Article |

    The charge-transfer characteristics of conjugated molecules are important in determining their electronic properties. Using resonant photoemission spectroscopy, Batraet al. quantify the through-space charge transfer in two model conjugated systems with femtosecond resolution.

    • Arunabh Batra
    • , Gregor Kladnik
    •  & Latha Venkataraman

  • Article
    | Open Access

    Achieving spin separation of charged particles in non-uniform magnetic fields is hindered by the Lorentz force. Kohdaet al. demonstrate spin separation in a semiconductor nanostructure by exploiting the effective magnetic field arising from the spin–orbit interaction and achieve highly polarized spin currents.

    • Makoto Kohda
    • , Shuji Nakamura
    •  & Junsaku Nitta

  • Article
    | Open Access

    A signature of the Dirac-like physics of charge carriers in graphene is the occurrence of an anomalous Hall effect, resulting in a quantization of the Landau levels. Guoet al. observe Landau levels of Dirac fermions in potassium-intercalated graphite arising in the absence of an applied magnetic field.

    • Donghui Guo
    • , Takahiro Kondo
    •  & Junji Nakamura

  • Article |

    The coil-globule transition undergone by polymers in solution delineates a transition from expanded coils to collapsed globules, depending on the polarity of the solvent. This study examines the influence of vibrational entropy on the transition, and finds it can induce a crossover from a second-order to a first-order transition.

    • Carlo Maffi
    • , Marco Baiesi
    •  & Paolo De Los Rios

  • Article |

    Ultrathin inorganic materials hold promise for a variety of applications, including flexible electronics. This work presents a fabrication method that permits the synthesis of large and flexible freestanding layers of zinc selenide that display a high-photocurrent density.

    • Yongfu Sun
    • , Zhihu Sun
    •  & Yi Xie

  • Article |

    One of the obstacles to improving the efficiency of organic photovoltaic solar cells is the recombination of polaron pairs at the interface between donor and acceptor molecules. By doping cells with galvinoxyl radicals, Zhanget al. demonstrate a mechanism that overcomes this problem via a spin-flip process.

    • Ye Zhang
    • , Tek P. Basel
    •  & Z. Valy Vardeny

  • Article |

    Charge stripe order has been predicted to be the ground state for the parent compounds of copper oxide superconductors. Using resonant X-ray diffraction, Schüßler-Lagenheineet al. probe the surface region of 12 percent doped La2−xSrxCuO4, and observe charge-stripe order.

    • H.-H. Wu
    • , M. Buchholz
    •  & C. Schüßler-Langeheine

  • Article |

    The torque contributions exerted by spin-polarized currents on magnetic structures are not fully understood due to the difficulty in discerning their relative weight. Pollardet al. propose a novel method to directly determine the value of the competing spin transfer torques by in-situLorentz microscopy.

    • S.D. Pollard
    • , L. Huang
    •  & Y. Zhu

  • Article
    | Open Access

    The optical transitions that occur in rare-earth-doped crystals offer promise for quantum information storage and processing. Kolesovet al.report the optical detection of a single praseodymium ion residing in a crystal host by using an excited-state absorption process to enhance its fluorescence yield.

    • R. Kolesov
    • , K. Xia
    •  & J. Wrachtrup

  • Article |

    Membrane-based technologies to separate oil–water mixtures are energy-intensive, suffer from fouling or cannot separate a wide range of mixtures. Now, a new membrane is reported that is superhydrophilic and superoleophobic, and can separate a range of oil–water mixtures with high efficiency, without an external energy source.

    • Arun K. Kota
    • , Gibum Kwon
    •  & Anish Tuteja

  • Article |

    The spectral position of Raman peaks is a useful diagnostic for determining the degree of strain and excess electronic charges present in graphene. This study demonstrates that these two contributions can be separated from each other and therefore be obtained at the same time.

    • Ji Eun Lee
    • , Gwanghyun Ahn
    •  & Sunmin Ryu

  • Article |

    Signal modulation is a mechanism which embeds an information-carrying signal into a carrier wave to broadcast information and is essential for high-speed communication. Zhonget al. report a flexible, transparent all-graphene modulator circuit performing quaternary modulation schemes with only two transistors.

    • Seunghyun Lee
    • , Kyunghoon Lee
    •  & Zhaohui Zhong

  • Article |

    Molybdenum disulphide offers some tantalizing advantages over graphene as a material with which to fabricate field-effect transistors. Kimet al. present a comprehensive study of field-effect transistors made from multilayer samples of MoS2and find that they can achieve high carrier mobilities.

    • Sunkook Kim
    • , Aniruddha Konar
    •  & Kinam Kim

  • Article |

    Singlet fission converts single singlet excitons into pairs of triplet excitons, and it has been proposed to give additional photocurrent to solar cells. Ehrleret al. use lead selenide nanocrystals of varying sizes to measure the triplet energy in pentacene photovoltaic cells, and achieve efficiencies approaching 5%.

    • Bruno Ehrler
    • , Brian J. Walker
    •  & Neil C. Greenham

  • Article |

    Understanding ultrafast demagnetisation is key to manipulating magnetic structures on fast timescales, yet laser sources limit the attainable spatial resolution. Here, a soft X-ray high harmonic source enables a high temporal and spatial resolution study of domain demagnetisation in [Co/Pt]30multilayer films.

    • Boris Vodungbo
    • , Julien Gautier
    •  & Jan Lüning

  • Article
    | Open Access

    Along with its electronic characteristics, the spin properties of graphene have recently received increasing attention in the context of spintronic applications. Using microwave radiation, Maniet al. identify resistively detected spin resonance in monolayer and trilayer graphene sheets and extract the value for the Landé g-factor.

    • Ramesh G. Mani
    • , John Hankinson
    •  & Walter A. de Heer

  • Article |

    Current-induced motion of magnetic nanostructures, such as skyrmions or domain walls, is envisioned as a promising scalable technology for information storage. Yuet al.demonstrate near-room-temperature motion of skyrmions with current densities orders of magnitude lower than previously reported in domain walls.

    • X.Z. Yu
    • , N. Kanazawa
    •  & Y. Tokura

  • Article
    | Open Access

    Quantum spin ice is a magnetic state of matter which can play host to monopole excitations. Using polarized neutron scattering, Changet al. show that the quantum spin ice material ytterbium titanate undergoes a Higgs transition of emergent magnetic monopoles from a Coulomb liquid to a ferromagnetic phase.

    • Lieh-Jeng Chang
    • , Shigeki Onoda
    •  & Martin Richard Lees

  • Article
    | Open Access

    Non-uniform light beams can create patterns in azo-polymer films by inducing mass transport, yet the process is not well understood. Using optical vortex beams, Ambrosioet al. observe the formation of spiral patterns that are surprisingly sensitive to the optical phase, which they explain with a new model.

    • Antonio Ambrosio
    • , Lorenzo Marrucci
    •  & Pasqualino Maddalena

  • Article |

    Topologically protected states of matter are receiving widespread attention owing to their unusual electronic properties. Using numerical simulations, this study predicts that tin telluride is a physical realization of a new class of materials termed topological crystalline insulators.

    • Timothy H. Hsieh
    • , Hsin Lin
    •  & Liang Fu

  • Article |

    Nacre is an organic–inorganic composite biomaterial, which consists of an ordered multilayer structure of crystalline calcium carbonate platelets separated by porous organic layers. Finnemoreet al. present a route to artificial nacre which mimics the natural layer-by-layer biosynthesis.

    • Alexander Finnemore
    • , Pedro Cunha
    •  & Ullrich Steiner

  • Article
    | Open Access

    Patchy colloids are colloidal particles with chemically or physically patterned surfaces that result in complex interactions arising between them. By means of numerical simulations, Romano and Sciortino show that suitably tailored patches can induce the crystallization of patchy colloids into specific crystal structures.

    • Flavio Romano
    •  & Francesco Sciortino

  • Article
    | Open Access

    The dynamics and structure of the glass transition in liquids is still debated. Using particle-level confocal microscopy, Leocmach and Tanaka investigate supercooled colloidal liquids and distinguish different scenarios for glassy slow dynamics, suggesting that local ordering may only play a minor role.

    • Mathieu Leocmach
    •  & Hajime Tanaka

  • Article |

    Vortex–charge duality is a model that has been proposed for describing the superconducting to insulator transition in disordered thin films. Mehtaet al. report experimental evidence for this duality in the two-dimensional electron gas that arises in LaAlO3/SrTiO3heterostructures.

    • M.M. Mehta
    • , D.A. Dikin
    •  & V. Chandrasekhar

  • Article
    | Open Access

    The iron pnictides are a class of superconductors that have received widespread interest in recent years. By doping the prototypical material LaFeAsO with hydrogen, this study reveals the existence of a second superconducting dome at higher doping ranges, which arises due to orbital fluctuations.

    • Soshi Iimura
    • , Satoru Matsuishi
    •  & Hideo Hosono

  • Article |

    Chiral metamaterials present interesting ways to manipulate and distinguish between different circular polarizations of light. Zhanget al. realize chiral metamaterials that exhibit photoinduced switching between left- and right-handed circular polarization interactions at terahertz frequencies.

    • Shuang Zhang
    • , Jiangfeng Zhou
    •  & Xiang Zhang

  • Article |

    The ability to manipulate single charges is a key requisite for novel nanoelectronic devices. Allenet al. show how to electrostatically confine electrons in suspended bilayer graphene quantum dots by local control of the graphene band structure.

    • M. T. Allen
    • , J. Martin
    •  & A. Yacoby

  • Article |

    The SrTiO3/LaAlO3 system is widely studied because it forms a two-dimensional electron gas at the interface. This study investigates the effects of diluting the LaAlO3 layer with SrTiO3, and finds that the threshold thickness required for the onset of conductivity scales inversely with the fraction of LaAlO3, suggesting an intrinsic origin for the electron gas.

    • M.L. Reinle-Schmitt
    • , C. Cancellieri
    •  & P.R. Willmott

  • Article
    | Open Access

    Switches made up of single molecules form the basis for the concept of molecular electronics. Miyamachiet al.demonstrate that an iron-based spin crossover molecule can be switched between different spin states, provided it is decoupled from a metallic substrate by a thin insulating layer.

    • Toshio Miyamachi
    • , Manuel Gruber
    •  & Wulf Wulfhekel

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