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| Open AccessShort hydrogen-bond network confined on COF surfaces enables ultrahigh proton conductivity
When hydronium ions are enriched in confined water, short hydrogen bonds (SHBs) form due to the constrained space of excess protons between pairs of water molecules. Here authors demonstrate a SHB network confined on the surface of ionic COF membranes with tunable -SO3H groups, with proton conductivity of 1389 mS cm-1 at 90 oC.
- Benbing Shi
- , Xiao Pang
- & Zhongyi Jiang
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| Open AccessMagnetic molecules as local sensors of topological hysteresis of superconductors
Magnetic molecules have long been seen to hold promise in magnetic sensing applications. In this paper, Serrano et al show that a single layer of a magnetic molecule, a terbium based complex, is sensitive to the local magnetic field variation of a superconducting surface on which it is deposited.
- Giulia Serrano
- , Lorenzo Poggini
- & Roberta Sessoli
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| Open AccessUltrafast transient liquid assisted growth of high current density superconducting films
High throughput manufacturing of long length coated conductors requires fast epitaxial growth of high-temperature superconducting films. Here, Soler et al. report an ultrafast growth rates and high critical current densities of YBa2Cu3O7 films using a transient liquid-assisted growth method.
- L. Soler
- , J. Jareño
- & T. Puig
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| Open AccessSynthesis of clathrate cerium superhydride CeH9 at 80-100 GPa with atomic hydrogen sublattice
Hydrogen-rich superhydrides are promising high-temperature superconductors which have been observed only at pressures above 170 GPa. Here the authors show that CeH9 can be synthesized at 80-100 GPa with laser heating, and is characterized by a clathrate structure with a dense 3-dimensional atomic hydrogen sublattice.
- Nilesh P. Salke
- , M. Mahdi Davari Esfahani
- & Jung-Fu Lin
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| Open AccessEmergent superconductivity in an iron-based honeycomb lattice initiated by pressure-driven spin-crossover
Up to now, all iron-based high-Tc superconductors contain a square iron lattice. Here, Wang et al. report the observation of superconductivity in an iron honeycomb lattice accompanied with pressure-driven spin-crossover, in-plane lattice collapse and insulator-metal transition.
- Yonggang Wang
- , Jianjun Ying
- & Ho-kwang Mao
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| Open AccessHigh-quality monolayer superconductor NbSe2 grown by chemical vapour deposition
Two-dimensional superconductors will likely have applications not only in devices, but also in the study of fundamental physics. Here, Wang et al. demonstrate the CVD growth of superconducting NbSe2 on a variety of substrates, making these novel materials increasingly accessible.
- Hong Wang
- , Xiangwei Huang
- & Zheng Liu
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| Open AccessChemical control over the energy-level alignment in a two-terminal junction
Energy alignment in molecular tunnelling junctions is desirable for altering their electrical properties, however controllability is still an issue. Here the authors report a 2 orders-of-magnitude increase in the tunnelling current via chemical control of the energy-level alignment at a two-terminal junction.
- Li Yuan
- , Carlos Franco
- & Christian A. Nijhuis
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| Open AccessThe microscopic structure of charge density waves in underdoped YBa2Cu3O6.54 revealed by X-ray diffraction
Near to the superconducting state, cuprates display spatially-periodic charge density variations. Here, the authors use x-ray diffraction to determine the microscopic structure, showing how charge density waves in underdoped YBa2Cu3O6.54break the symmetry of the superconducting layers.
- E. M. Forgan
- , E. Blackburn
- & S. M. Hayden
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| Open AccessLocal destruction of superconductivity by non-magnetic impurities in mesoscopic iron-based superconductors
The pairing symmetry of the wavefunction in high-Tciron-based superconductors remains not completely understood. To shed light on this problem, here the authors investigate the local destruction of superconductivity by introducing Zn impurities in the BKZn iron arsenide compound.
- Jun Li
- , Min Ji
- & Victor V. Moshchalkov
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| Open AccessDirect characterization of photoinduced lattice dynamics in BaFe2As2
In BaFe2As2, the lattice couples strongly to the magnetic and electronic degrees of freedom, providing a way to control them. Here, by means of time-resolved X-ray scattering, the authors measure rapid lattice oscillations, which can induce changes in the material’s electronic and magnetic properties.
- S. Gerber
- , K. W. Kim
- & W.-S. Lee
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Anomalous magnetoresistance in the spinel superconductor LiTi2O4
LiTi2O4is the only known spinel oxide superconductor, but systematic investigations of its transport properties have been lacking so far. Here, the authors' analyses detect an unusual magnetoresistance, revealing spin-orbit fluctuations similar to those in high-temperature superconductors.
- K. Jin
- , G. He
- & I. Takeuchi
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Berry phases and the intrinsic thermal Hall effect in high-temperature cuprate superconductors
A fully quantum mechanical description of the thermal Hall effect in high-temperature cuprate superconductors remains elusive. Here, by connecting it to momentum space Berry phases, the authors calculate the dependence of the intrinsic thermal Hall conductivity on temperature, external field and pairing gap.
- Vladimir Cvetkovic
- & Oskar Vafek
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| Open AccessAnomalous critical fields in quantum critical superconductors
Superconductivity in the iron pnictides is believed to be related to quantum critical fluctuations. Putzke et al. observe unexpected anomalies in the critical fields of BaFe2(As1−xPx)2that emerge close to its magnetic critical point, which they argue is a generic feature of quantum critical superconductivity.
- C. Putzke
- , P. Walmsley
- & A. Carrington
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High-energy spin and charge excitations in electron-doped copper oxide superconductors
Understanding spin dynamics in the cuprates is vital to understanding the origin high-temperature superconductivity. X-ray and neutron spectra obtained by Ishii et al.suggest that the spins in electron-doped cuprates are itinerant, in contrast to recent evidence that in hole-doped cuprates they are localized.
- K. Ishii
- , M. Fujita
- & J. Mizuki
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Spin waves and magnetic exchange interactions in insulating Rb0.89Fe1.58Se2
Unlike the other iron-based superconductors, the parent compounds of the alkaline iron selenide superconductors are insulators. Dai and colleagues examine the spin-wave excitations in these materials and uncover evidence for a common magnetic origin for all iron-based superconductors.
- Miaoyin Wang
- , Chen Fang
- & Pengcheng Dai
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Superconductivity at 5 K in alkali-metal-doped phenanthrene
Intercalating alkali metals into picene—a hydrocarbon with five linearly fused benzene rings—results in superconducting materials. Now, alkali-metal-doped phenanthrene, which consists of three fused benzene rings, is also found to be superconducting, opening up a broader class of organic superconductors.
- X.F. Wang
- , R.H. Liu
- & X.H. Chen
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| Open AccessAdvantageous grain boundaries in iron pnictide superconductors
High critical temperature superconductors could be used to produce ideal electric power lines, but the misalignment of crystalline grain boundaries reduces current density. Here, pnictide superconductors are found to be more tolerant to misaligned grain boundaries than cuprates.
- Takayoshi Katase
- , Yoshihiro Ishimaru
- & Hideo Hosono
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| Open AccessProximity of iron pnictide superconductors to a quantum tricritical point
In some iron-based materials, unconventional superconductivity can emerge near a quantum phase transition where long-range magnetic order vanishes. Giovannettiet al.show that the magnetic quantum phase transition in an iron pnictide superconductor is very close to the quantum tricritical point.
- Gianluca Giovannetti
- , Carmine Ortix
- & José Lorenzana
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Pseudogap in a thin film of a conventional superconductor
In high-temperature superconductors, a very low density of states, the pseudogap, exists even above the critical temperature. Here, the authors show that this is also the case for a conventional superconductor, titanium nitride thin films, and that this pseudogap is induced by superconducting fluctuations.
- Benjamin Sacépé
- , Claude Chapelier
- & Marc Sanquer
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| Open AccessAnisotropic structure of the order parameter in FeSe0.45Te0.55 revealed by angle-resolved specific heat
The structure of the superconducting gap of iron pnictide superconductors is controversial. In this paper, angle-resolved specific heat measurements are used to show that the gap is anisotropic, which is consistent with an extended s-wave model of superconducting pairing.
- B. Zeng
- , G. Mu
- & H.-H. Wen