Introduction

Optical frequency combs (OFCs) have been identified as a key building block for many applications ranging from spectroscopy1,2 and lidar3 to optical communications4,5,6. The ubiquity and versatility of frequency combs naturally made them a crucial field of research, especially in photonics as tremendous performances can be reached thanks to the intrinsic advantages of light and light technology. Several photonic techniques and platforms have been demonstrated for generating frequency combs covering the visible to the THz spectral range7,8,9,10,11. Combined with the progress of photonic integration, highly compact, relatively cheap, energy-efficient combs sources are now accessible12,13,14. There is, however, an inherent trade-off between current OFC sources: large comb bandwidths typically come at the price of no or limited tunability, meaning that a system tends to be optimized for one specific use case. In this sense, having a single device with the ability to tune the comb spacing or control the spectral envelope or even the coherence would be highly desirable so that one system could match the requirements of various applications. We identify four parameters of OFC sources whose tunability would be a strong plus: 1) The free-spectral range (FSR), i.e. the spectral comb line spacing, e.g. for flexible grid transmission networks15,16,17. 2) The frequency comb centre wavelength, e.g., for spectroscopy applications18. 3) The frequency envelope, to direct all the power to the frequency range of interest, e.g., for THz generation19. 4) The coherence of the comb lines, e.g., for lidar or ranging applications for which broad linewidth can aid absolute positioning20. Different approaches have been considered to adjust the properties of the OFC. One can start from a broad frequency comb and process it to achieve the desired features. The envelope of the comb can relatively easily be tuned with frequency filters, but the FSR is fixed by the initial comb source. For instance, mode-locked lasers and micro-cavities generate broadband combs with excellent properties, but the corresponding FSR is intrinsically fixed21 and small FSR values, typically below the GHz, represent a challenge with these approaches. On top, optical filters also suffer from limited bandwidth, and centre frequency control requires complex setups, hindering photonic integration22,23,24,25. Even more importantly, the power of filtered frequencies is totally lost. On the other hand, nonlinear approaches to perform more advanced comb processing or conversion tasks are promising and flexible but are typically energy inefficient as they require high power input26. Alternatively, electro-optic (EO) comb sources are more straightforward and flexible, but they are facing major limitations in terms of frequency range: reaching mm-wave frequencies is already an issue, thus keeping most of the THz range out of reach for now. To overcome these hurdles, one requires complex systems and techniques such as cascading EO phase-modulator devices together with highly nonlinear fibers27 or microresonators28. Last, recent works showed the potential of optical injection schemes in semiconductor lasers to unlock comb processing capabilities. Injecting an optical frequency comb into a semiconductor laser can lead to comb broadening and changes in the polarization properties of the comb29,30.

In this work, we demonstrate frequency-agile spectral multiplication of an EO-comb by a semiconductor multi-wavelength laser (MWL). Our novel scheme combines the flexibility of the EO-comb with the large bandwidth of a multi-wavelength laser to obtain a versatile OFC with a flexible spectral envelope over THz-range frequencies. Through optical injection of a narrowband comb, we achieve comb multiplication from tens of GHz up to 1.3 THz, while preserving the RF coherence of the injected comb, i.e. the phase correlation between its comb lines. However, phase correlation between the various sub-combs is not achieved per se. As such, we refer to this process as spectral multiplication rather than comb broadening. We further demonstrate that the different multiplied combs can be turned on and off on demand with over 30 dB side-mode suppression ratio. The control mechanism is realized by adjusting the phase in a tailored optical feedback cavity monolithically integrated with the laser, allowing switching at the nanosecond time scale. Moreover, we show that phase locking between the multiplied combs can be achieved either by adding an extra tone to the injected signal or carefully adjusting the tone spacing of the injected comb, thus leading to “cascaded” phase locking of neighboring combs. Finally, we report an excellent agreement with numerical simulations based on a multi-mode rate equation model. Besides reproducing the experimental results, our numerical investigations highlight the crucial importance of the coupling between the different wavelengths of the MWL to enable spectral multiplication. This work represents a novel direction towards high-speed versatile on-chip optical processing of optical signals, not only limited to frequency combs, over THz spectral ranges.

Results

THz-scalable spectral multiplication of a frequency comb with an on-chip MWL

The concept we propose for on-chip comb spectral multiplication with an integrated multi-wavelength laser (MWL) is depicted in Fig. 1. The inherent emission of the MWL consists of multiple modes (λ1, λ2, …, λn) which can be flexibly designed to be spectrally separated from a few GHz to several THz; the main limit being the gain bandwidth of the associated active medium, e.g., up to 10 THz around 1550 nm in the InP platform31. A control mechanism enables emission at a specific λn or even at multiple wavelengths, e.g., λn and λm, simultaneously. To achieve spectral multiplication, a narrow comb, i.e., with a bandwidth of a few GHz to tens of GHz, is injected around one of the suppressed modes of the MWL. Owing to the intrinsic coupling between the modes of the MWL, the injected comb is spectrally multiplied around the different wavelengths emitted by the MWL. Similarly, the control mechanism of the MWL allows for selecting around which wavelength(s) the spectral multiplication will take place, thereby modifying the envelope of the output comb. Due to the fast response of the laser, switching between different wavelengths can be achieved at the nanosecond timescale. Such a THz-range spectral multiplication of narrowband frequency combs allows for energy-efficient and programmable spectral control over a THz range, which can be adjusted at nanosecond (GHz) speeds advantageous for, e.g., spectroscopy applications, THz generation, or even flexible networks.

Fig. 1: THz-range frequency comb spectral multiplication with a multi-wavelength laser (MWL).
figure 1

A narrowband frequency comb is spectrally multiplied to frequency offsets ranging from tens of GHz to few THz by injecting it in a controllable integrated multi-wavelength laser (MWL) photonic chip. Without optical injection, the MWL can be controlled to emit at wavelengths λ1, λ2, …, λn. High-speed mode switching at nanosecond time scales is achieved by adjusting a single control parameter X. Under frequency comb injection, the inherent mode coupling in the MWL leads to frequency comb multiplication at around the MWL emission wavelengths. By adjusting the control parameter, switching between GHz-range and THz-range frequency comb spectral multiplication can be achieved at nanosecond time scales.

Demonstration of comb multiplication up to 1.3 THz in a dual-cavity laser

The backbone of the proposed spectral multiplication technique is a multi-wavelength laser combined with the optical injection of a frequency comb. In this work, the MWL is a dual-cavity laser with two detuned distributed Bragg reflectors (DBR) placed in a row, a shared semiconductor optical amplifier (SOA), and a broadband reflector (BR), see Fig. 2a, and refer to the Methods for a detailed description of the photonic integrated circuit. The DBRs are detuned by approximately 10 nm (1.3 THz) with corresponding Bragg wavelengths at approximately 1537 nm and 1547 nm. While the laser was initially optimized to emit at two distinct wavelengths with 10 nm separation, multiple longitudinal modes can emit around each DBR’s Bragg wavelength depending on the current sent to the DBRs. In this work, we use the term ”mode” to refer solely to these longitudinal modes. The laser threshold current is at 21 mA, and we operate at ISOA1 = 30 mA. In this configuration, see Methods, the free-running laser emits at λ4 = 1547.58 nm, a longitudinal mode corresponding to the cavity defined by DBR2. Three additional residual modes can be observed at λ1 = 1536.70 nm, λ2 = 1536.92 nm, and λ3 = 1537.13 nm, corresponding to the cavity defined by DBR1. These modes are suppressed by more than 30 dB compared to the power of the dominant mode, see Section 1 of the Supplementary Information. The optically injected signal consists of a frequency comb featuring 5 tones with an FSR of 1 GHz. Multi-wavelength emission requires a careful gain balance between all emitted modes, but, from this point of view, optical injection represents a major disturbance. Thus, to avoid switching off un-injected modes when the optical injection is added, we inject the comb around λ3 that is strongly suppressed in the free-running configuration. This way we can achieve so-called partial-locking, i.e. the other modes are still on, despite sending a relatively strong injection signal32. When the injection signal is powerful enough and the detuning, defined as the frequency difference between the central peak of the comb and the injected wavelength, is small enough, the multi-wavelength laser re-generates the comb around the injected wavelength, see Fig. 2(b). We set the detuning and the injection strength to Δ = 2.3 GHz and κinj = 9.5 dBm, respectively. Here, we define the injection strength as the optical power of the injected signal at the lensed fiber (LF) input. It is important to note that the injection strength and the detuning have a visible effect on the laser output, for more details see Section 2 of the Supplementary Information. With the frequency comb being picked up by λ3, spectral multiplication of the modulated signal at λ4 is obtained through the modulation of the carrier population. Because the injected mode experiences amplitude modulation induced by the frequency comb, the carrier population of the laser will experience similar fluctuations. Then, due to the carrier coupling between all modes of the MWL, frequency combs emerge at the other wavelengths emitted by the MWL, in this case, λ4. We thus obtain multiplied combs separated by up to 1.3 THz. Depending on the laser configuration, we can multiply the frequency combs to different frequency offsets from a few GHz up to a few THz, depending on the mode emitted by the MWL. Although a similar behavior has already been reported in other laser systems29, this is the first time, to the best of our knowledge, that this effect is triggered across such a large frequency offset.

Fig. 2: THz-range agile frequency comb spectral multiplication using a feedback-controlled semiconductor MWL.
figure 2

a Experimental setup. To generate the EO-comb, the light from an external cavity laser (ECL) is sent through a Mach-Zehnder modulator (MZM, Vπ ≈ 6 V) driven by an arbitrary waveform generator (AWG). The polarization and strength of this injected signal is adjusted with a polarization controller (PC) and an EDFA, respectively. The light is coupled in and out of the photonic integrated circuit (PIC) containing the MWL with feedback cavity via a lensed fiber (LF). A high-resolution (5 MHz RBW) optical spectrum analyzer (OSA) records the output spectrum. An optical bandpass filter (BPF) followed by a high-speed photodiode (40 GHz BW) is used to select a sub-comb which is then analyzed by an electrical spectrum analyzer (ESA). b Optical spectrum of the re-generated and multiplied combs when the feedback is off (ISOA2 = 0 mA) and the narrowband comb is injected around λ3. The dashed lines indicate the wavelengths λ1 to λ4 of the residual longitudinal modes of the MWL. Without feedback, the frequency comb is multiplied at around λ4. c Optical power of the various sub-combs as a function of the voltage, VEOPM, applied to the EOPM for ISOA2 = 21 mA and comb injection around λ3. Comb switching occurs between the multiplied combs at around λ1, λ2, and λ4. d Optical spectral for various VEOPM values: V1 = 0 V, V2 = 3 V, V3 = 4.6 V, V4 = 7 V, and V5 = 8 V. e RF spectrum of the resulting beating between the tones of each comb (multiplied and re-generated). The low ( < 1 Hz) linewidth, limited by the RBW of the ESA (1 Hz), shows that the coherence of the injected comb is preserved after the injection.

Frequency-agile spectral multiplication through optical feedback control

While spectral multiplication is interesting in itself, e.g., for spectral shaping of frequency combs, it also offers an exciting opportunity in terms of tunability which is a crucial point to enable versatile technological solutions. Here, we rely on weak optical feedback from a monolithically integrated feedback cavity that simply comprises a semiconductor optical amplifier (SOA) to control the feedback strength and an electro-optic phase modulator (EOPM) to control the feedback phase, see Fig. 2(a). In previous work, we showed controllable switching between different wavelengths emitted by our MWL33. The switching mechanism is primarily based on a careful design of the feedback cavity length, which should ensure that the different modes are sent back towards the laser in anti-phase, roughly acting like a Fabry-Perot interferometer. Tuning the feedback phase then allows us to select which wavelength is resonant in the external cavity. This approach works well to control more than two modes in the laser cavity34, even with a design initially optimized for two specific wavelengths. The feedback phase is controlled by applying a voltage VEOPM to the EOPM (Vπ ≈ 12 V) of the feedback cavity. We set the feedback strength by driving SOA2 with ISOA2 = 21 mA, and keep the injection current of the MWL at ISOA1 = 30 mA, as previously. Without optical injection, such feedback control enables switching between three modes of the MWL at λ1, λ2, and λ4. In this case, the mode at λ3 remains strongly suppressed for any VEOPM value, which is why we inject the frequency comb around λ3. When EO-comb injection is present, we observe similar switching performances. As a result, by simply tuning the phase of the optical feedback cavity we can switch between three different multiplied combs. The re-generated comb which is emitted around the injected mode always remains present, see Fig. 2(c), which shows the evolution of the power for each comb when VEOPM is varied from 0 V to 8.5 V. Below 1 V, the comb is multiplied to the first longitudinal mode of the first cavity at λ1. Close to 1 V, the comb at λ4 starts emitting leading to comb switching from λ1 to λ4. For VEOPM > 5 V, emission around the second longitudinal mode of the first cavity, at λ2, is gradually switched on while emission at λ4 is turned off. While the first transition from λ1 to λ4 occurring for VEOPM ≈ 1 V appears to be rather sharp, the second transition from λ4 to λ2 is significantly smoother with the two combs appearing simultaneously in a small range of voltages around VEOPM ≈ 5 V. Note that, without injection, the laser exhibits similar switching behavior between λ1, λ2, and λ4, see Section 1 of the Supplementary Information. Figure 2(d) depicts the spectral multiplication of the injected frequency comb at different VEOPM values. In this MWL configuration, we achieve sequential emission of three multiplied combs in the mm-wave and THz range with an FSR of 1 GHz and central frequencies around 26 GHz, 54 GHz, and 1.3 THz, as shown in cases V4, V1, and V2 in Fig. 2(d), respectively. We achieve an extinction ratio, i.e., power difference between the on and off state, for each multiplied comb, of above 30 dB, only relying on phase-controlled optical feedback. The peak power of the multiplied combs, measured just after the lensed fiber, is between -12 dBm and -13 dBm, comparable to the optical power of -11 dBm of the comb generated around the injected wavelength. With careful tuning of the feedback phase, the simultaneous emission of two multiplied combs, e.g., at λ2 and λ4, can be achieved, see case V3 in Fig. 2(d). While changing VEOPM, we observe that the center wavelength of both the re-generated and multiplied comb remains stable with variations of ± 100 MHz for the multiplied combs, based on optical spectra measurements with limited absolute accuracy. Similarly, the comb bandwidth and shape are overall well preserved with only small variations. In particular, we measure bandwidths of up to 10 GHz for both the re-generated and multiplied combs. We can therefore conclude that, besides the wavelength switching, the impact of the feedback on the comb generation process is limited. This is an important point as it suggests that the two processes - optical injection and optical feedback - could potentially be analyzed and optimized rather independently.

An important added value of this control technique is the speed. The EOPM has a large bandwidth of up to several tens of GHz even on generic foundry platforms35. Besides, the laser is effectively switching between two different states which are both above the threshold: the carrier population is already filled in and the feedback only leads to small gain variations. As a result, even without proper RF optimization, we achieve switching times below 4 ns, further details are given in Section 4 of the Supplementary Information. We believe that these performances could be further improved by using co-planar waveguide transmission lines and electrical isolation of the EOPM. Regarding the characteristics of the sub-combs, we observe that, while the re-generated and multiplied combs feature different bandwidths depending on the MWL and injection parameters, the RF linewidth of the original EO-comb is preserved. We confirm it experimentally by isolating sub-combs using an optical filter and analyzing their respective RF spectrum using a photodiode (PD) and an electrical spectrum analyzer (ESA). Fig. 2e depicts the resulting tone centered at 1 GHz featuring a sub-Hz linewidth, limited by the ESA resolution bandwidth. There is, however, only a limited phase correlation between the different combs emerging at different wavelengths. We confirm it by isolating the two neighboring sub-combs for VEOPM = 7 V, at around λ2 and λ3, see Fig. 3a. The resulting RF spectrum, Fig. 3b, features a broad beatnote at around 25 GHz with a long-term 3-dB-linewidth of 38 MHz, indicative of the lack of coherence between the sub-combs. In the following section, we further discuss how to achieve phase correlation between the various sub-combs.

Fig. 3: Phase correlation between sub-combs.
figure 3

a Optical spectrum of the sub-combs centered at around λ2 and λ3. The large difference in optical linewidth between the tones of the two sub-combs is indicative of the lack of coherence between the sub-combs. b RF spectrum of the photomixed sub-combs. The strongest beatnote features a long-term 3-dB-linewidth of approximately 38 MHz, linked to the absence of coherence between the sub-combs.

Cascaded phase-locking of multiplied combs

Unlike the tones of each re-generated or multiplied comb, the different wavelengths (λ1, λ2, …, λn) emitted by the MWL are not inherently phase-locked nor phase-correlated. This means that the different sub-combs are actually not phase-correlated with one another. The RF linewidth of the tones obtained from the beating of two sub-combs is several MHz, matching the typical laser linewidth of the MWL. Yet, various techniques could be employed to phase-correlated the sub-combs, e.g., exploiting four-wave mixing (FWM) effects in SOA36, thereby achieving comb broadening. We discuss here two different approaches leading to the phase-locking of the multiplied combs. The first one consists of adding an extra tone to the modulated optical injection on top of the EO comb already present. The extra tone is directly added using the AWG, see Fig. 4a–c. When this extra tone is close to an active mode of the MWL, the multiplied comb can then be actively phase-locked to the re-generated comb. This approach is illustrated in Fig. 4d–f considering the same laser configuration and feedback detailed in the previous subsection, though we only focus on the longitudinal modes belonging to the laser cavity defined by DBR1. Without injection and with ISOA2 = 21 mA and VEOPM = 0 V, λ1 is dominant and the other longitudinal modes, λ2, and λ3 are strongly suppressed as shown in Fig. 4d. The EO-comb signal is injected around λ3, while the extra tone which is phase-locked with the EO-comb is injected around λ2, at an offset frequency ftone from the center of the comb. The EO-comb injection triggers the OFC re-generation at wavelength λ3 while the extra tone triggers a multiplied comb around λ2, see Fig. 4e. We isolate the two combs emerging around λ2 and λ3 with a bandpass filter (BPF-I) and impinge the light into a PD followed by an ESA. We record the resulting spectrum with the ESA and observe an RF comb centered at around 26 GHz with the associated tones featuring linewidths below 1 Hz confirming an excellent phase correlation. Adding an extra tone in the injected comb, therefore, appears to be an effective way to force phase-locking between the re-generated and neighboring multiplied combs. It can however quickly become challenging as the wavelength difference increases and could even be out of reach for frequency differences in the THz as demonstrated earlier in this paper.

Fig. 4: Coherence control through cascaded phase locking.
figure 4

a Experimental setup: A narrowband optical frequency comb with an extra tone is generated by modulating the light from an external-cavity laser (ECL) with a Mach-Zehnder modulator (MZM) driven by an arbitrary waveform generator (AWG). b Optical spectrum of the narrowband frequency comb with 1 GHz FSR. c Optical spectrum of the combined narrowband 1-GHz-FSR comb and side tone at a frequency difference ftone with respect to the center of the comb. d Optical spectrum, before injection, of the longitudinal modes associated with the long cavity of the MWL defined by DBR1. e Optical spectrum of the MWL output under comb injection around λ3 and ftone = 26.1 GHz. The spectrum shows the re-generated and multiplied combs at around λ3 and λ2, respectively. At such ftone value, the extra tone is injected around λ2, leading to comb multiplication around λ2. f Optical spectrum of the re-generated and multiplied combs at well-tuned ftone of 26.2 GHz. Accurate optimization of the offset of the extra tone leads to cascaded phase locking of the multiplied comb emitting around λ1. g RF spectrum resulting from the beating of the re-generated and multiplied comb for ftone = 26.1 GHz. The inset indicates the narrow linewidth ( < 1 Hz) of the beating at the highest resolution bandwidth (RBW) of our ESA (1 Hz). h Averaged optical linewidth, measured at 10 dB, of the tones from the comb at λ1 as a function of ftone. The red dashed line at 5 MHz depicts the RBW limitation of the OSA. i RF spectrum resulting from the beating of the two multiplied combs for ftone = 26.2 GHz. The inset indicates the narrow linewidth ( < 1 Hz) of the beating at the highest RBW of our ESA.

On the other hand, we also show that a careful tuning of the frequency ftone of the extra tone can trigger the emission of a second multiplied comb, phase-locked to the two other combs, around λ1. When the frequency of the extra tone ftone is changed, the power, bandwidth, and linewidth of the comb emitting around λ1 vary significantly. At well-optimized frequency offsets, the second multiplied comb at around λ1 experiences a major linewidth reduction and power amplification. Figure 4(h), depicts the average value of the long-term 10-dB optical linewidth37 of the comb lines emitting around λ1, as a function of the ftone, measured with an optical spectrum analyzer (OSA) with a resolution bandwidth of 5 MHz. The linewidth reduction occurs sharply for ftone values ranging from 26.14 GHz to 26.26 GHz. To accurately measure the phase correlation between the two multiplied combs around λ1 and λ2, we isolate them using a bandpass filter (BPF-II) and send the output to a PD followed by an ESA. Figure 4(i) depicts the resulting RF spectrum for ftone = 26.2 GHz. The RF spectrum contains a frequency comb centered at the beat note frequency between the two OFCs, with each tone featuring a linewidth below the resolution limit of 1 Hz of our ESA. Outside the optimized range, the RF spectrum depicts broadband noise, see Section 5 of the Supplementary Information. These tones are generated from the beating between comb lines of the two multiplied combs, therefore, by fine-tuning the frequency offset of the extra tone we can achieve a phase correlation between the three neighboring combs. We were not able to observe a similar feature with the multiplied comb emitting around λ4 with a 1.3 THz separation from the injected comb, with the current configuration between the modes of our MWL. One interpretation is linked to the interaction between the re-generated and phase-locked multiplied combs, which leads to a modulated comb appearing at their beating frequency. By tuning the frequency offset, ftone, the resulting modulation caused by the beating can be locked on the first mode λ1 which is not directly affected by the injection. In other words, the interaction between the two neighboring combs leads to a cascaded phase locking of the modes. We believe that cascaded phase-locking can advantageously be extended to additional modes leading to even larger frequency differences, although we could not find a suitable configuration to test it experimentally.

Numerical model and simulations: impact of the mode coupling parameter

Looking at the dynamical behavior of semiconductor lasers, rate equation models, despite their simplicity, have been shown to qualitatively predict most if not all, dynamical features reported experimentally. In addition, their simplicity allows the use of advanced techniques such as continuation to further clarify the nonlinear mechanisms at play. Here, we use a phenomenological multi-mode model initially derived for solid-state lasers but adapted for semiconductor lasers38. We have extended this model to include optical frequency comb injection and optical feedback to match our experimental scheme, see Methods. Considering the complexity of the coupling mechanism - represented here by the cross-saturation between each mode pair - and that the number of parameters describing such coupling quickly increases with the number of modes, we report here results obtained for two-mode model only, while in Section 7 of the Supplementary Information, we report results for the three-mode model. Using typical semiconductor laser parameters, comb multiplication can be easily obtained providing that the gain balance and mode coupling parameter between the different modes have been adjusted to allow for simultaneous emission of both the re-generated and multiplied combs32. Similarly, feedback-induced switching between the multiplied combs is well reproduced qualitatively as shown in Section 7 of the Supplementary Information. In fact, the main unknown is the value of the cross-saturation parameter β and its impact on the comb generation mechanism. To bring new insight into this question, we have explored the parameter space for a two-mode model for different values of the mode coupling parameter β as pictured in Fig. 5. An important aspect to consider is that cross-saturation influences the power balance between the modes. To keep the same balance, which is crucial in the use case considered here, we need to carefully adjust the modal gain after changing the cross-saturation parameter32. We use this approach to analyze the effect of changing the coupling strength between modes while keeping all other parameters, except the modal gain, fixed. We adjust the parameters to obtain a 40 dB suppression ratio between the dominant and suppressed mode, similar to experimental observations. Next, we add an injection of an optical frequency comb with 5 tones to the suppressed mode, see Methods.

Fig. 5: Numerical investigation of the impact of the cross-coupling parameter β on the frequency comb multiplication for a two-mode model, i.e., dual-wavelength laser.
figure 5

The laser dynamics acquired for β = 0.95 are presented for the injected (a) and un-injected (b) modes. Similarly, the dynamics obtained for β = 0.88 are illustrated for the injected (c) and un-injected (d) modes. For each line, panel (1) displays the κinj-Δ map of the bandwidth of the output signal emerging around both the injected (a, c) and un-injected (b, d) modes. Panel (2) represents the κinj-Δ map of the total power of the output signal, while the black dots in panel (3) show where the FSR estimated from the output signal doesn't match the FSR of the injected comb, thus indicating a different type of dynamics. Spectra of the output signal emerging around the injected (a.4, a.5) and un-injected (b.4, b.5) modes for two sets of κinj and Δ values indicated by the triangles and the rectangles in the κinj-Δ maps where β = 0.95. The triangle is located within the locking range (shown by red dashed line), while the rectangle resides outside the locking range within the positive detuning values. The locking range is computed without modulation and for a CW injection. Spectra of the output signal emerging around the injected (c.4, c.5) and un-injected (d.4, d.5) modes for two sets of κinj and Δ values at β = 0.88. The two sets of parameters are depicted by diamonds and stars within and outside the locking range, respectively.

As already reported by others32,39, we observe that the injection parameters have a strong impact on the comb generation process for both injected and un-injected modes. For positive detuning values, on the right side of the locking region in Fig. 5, spectral multiplication appears, exemplary spectra of both the re-generated and multiplied comb are depicted in panel (4) and (5) of Fig. 5. Note that the locking range is defined for CW optical injection and it is shown by red dashed line. Moreover, the power balance between the re-generated and multiplied combs can be easily adjusted by tuning either the injection strength or the detuning. For negative detuning values, we observe a small region showing broad comb bandwidth for both the re-generated and multiplied comb, but it is also where different dynamical behavior is typically observed. To estimate the FSR of the output signal, we consider the signal with spectral components surpassing a predefined threshold. Subsequently, we calculate the separation between the different spectral components of the output signals. In panel (3) of Fig. 5, the presence of black dots signifies areas where the separation between the spectral components of the output signal does not match the FSR of the injected comb, indicating different dynamical behavior for both modes, see Section 6 of the Supplementary Information. Although we did not perform such a systematic investigation experimentally, these features are well in line with our observations. Investigating the impact of the coupling parameter, we mainly see that the locking region is shrinking, pushed towards stronger injection when the coupling is decreased, see Fig. 5c and d. Different dynamical behaviors also appear to be partially inhibited when decreasing the coupling parameter. Interestingly, with respect to the locking range, the regions where spectral multiplication, suppression of the multiplied comb, and dynamics occur are preserved. That is, additional dynamics occur at negative detuning values, suppression of the multiplied comb occurs within the locking range, while spectral multiplication with large comb bandwidths occurs at the positive detuning side of the locking range. In particular, we foresee promising configurations emerging for weak injection and slightly negative detuning where much larger comb bandwidths appear. Our numerical investigations, therefore, suggest that weaker coupling between wavelengths might be desirable in the context of spectral multiplication. However, the wavelength coupling remains to be properly quantified experimentally, while its actual impact still needs to be investigated in detail.

Discussion

We have shown the potential of multi-wavelength lasers to achieve spectral multiplication of optical frequency combs in a flexible and efficient way. We demonstrate spectral multiplication over more than 10 nm (1.3 THz) with adjustable frequency through a single control parameter. A key advantage of our approach is that it is scalable in frequency, with the fundamental limitation being the bandwidth of the gain medium. Yet, for the generic foundry InP integration platform used, lasers with a tuning range over 75 nm (approximately 10 THz at 1550 nm) have already been reported40. In addition, complete integration of our system on a single photonic integrated circuit is well within reach as commercial generic foundry platforms already provide phase modulators with more than 25 GHz bandwidth directly in their standard process (and even > 50 GHz for electro-absorption modulators41). Secondly, we confirm that tailored phase-controlled optical feedback can be efficiently used to control multi-wavelength lasers even under optical frequency comb injection. We demonstrate that weak feedback allows tuning the power balance between the different modes of the MWL without disrupting the internal mode competition on which we rely for spectral multiplication. In addition, unlike other schemes relying on strong feedback forcing to achieve switching - e.g., using internal frequency filters42 or the so-called extended cavity regime31,43 – we expect to have a significantly lower requirement in terms of power for the optical injection signal. Finally, while there is no phase-locking between the different wavelengths of our MWL – only a noise correlation already identified as an important added value for high-frequency signal generation44 – we show that the addition of an extra tone in the injected EO-comb can trigger a cascaded mechanism leading to phase-locking of neighboring longitudinal modes. From an application viewpoint, it could benefit all use cases of frequency combs for which additional flexibility and programmability of the comb parameters are needed, but also applications where the extension of high-quality combs towards THz frequency is required. Our results show that it is possible to control the emission of the MWL thereby enabling THz-range frequency comb multiplication. When combined with THz photomixers, these chip-scale devices would enable compact, low-cost sources for programmable THz comb generation which could allow for ultra-high speed wireless communications (for 6G and beyond) and spectroscopy of biomolecules. Alternatively, the proposed spectral multiplication scheme could bridge the gap between narrowband low-FSR combs45,46 and broadband large-FSR combs28,47. Indeed, our approach has the potential to drastically extend the current capability to select the best of both worlds by copying the properties of the dense comb while maintaining the coherence provided by the broad comb.

Methods

Photonic integrated circuit design: dual-cavity laser with phase-controlled optical feedback

The multi-wavelength lasers (MWL) monolithically integrated with the optical feedback cavity have been fabricated on the InP generic foundry platform of SMART Photonics41. The detailed structure is schematically described in Fig. 2a. The design only uses the standard building blocks of the platform. The laser is a dual-cavity laser composed of a broadband two-port multimode interference reflector (BR, 40% reflectivity), a 500 μm-long semiconductor optical amplifier (SOA), and two distributed Bragg reflectors (DBRs) with a length of L1 = 500 μm and L2 = 250 μm, respectively. The DBRs are arranged sequentially and act as wavelength-selective elements. The pitch of the DBRs is set to 0.236 μm and 0.234 μm for DBR1 and DBR2 respectively, leading to roughly 10 nm spectral separation between the two cavity modes. The laser consists of two cavities with a length of 1396.26 μm and 1082.43 μm corresponding to DBR1 and DBR2, respectively. The MWL is coupled to an external cavity via an 85/15 multimode interference (MMI) splitter, meaning that only 15% of the light is sent toward the feedback cavity. The external cavity is composed of a 300 μm-long SOA, an electro-optic phase modulator (EOPM), and a one-port broadband reflector (BR) with 80% reflectivity. The total length of the external cavity is approximately 2.42 mm thus corresponding to the so-called ”short-cavity regime”. At SOA transparency, assuming all other components are ideal, we estimate that approximately 1.8% of the light is fed back toward the MWL cavity. The EOPM is designed to introduce a phase shift of π when biased at approximately 12 V, i.e., 2π for a total round trip in the feedback cavity. Further details on the laser and cavity designs can be found in Ref. 33. Both MWL and OFB are implemented on the same chip which is electrically packaged with all-metal pads being wire-bonded to PCB boards. In addition, it has been glued on a Peltier element including a thermistor. During our experiments, the temperature of the chip is set to 22 C.

Experimental setup for comb multiplication

The injected electro-optic (EO) comb is generated by a high-quality tunable laser (Keysight N7776C) whose optical output is then modulated by a LiNbO3 Mach-Zehnder modulator (MZM, IxBlue MXAN-LN-40, 40 GHz bandwidth, Vπ = 6 V). Electric signal modulation is generated by an arbitrary waveform generator (AWG, Keysight M8194A) and sent to the RF port of the MZM. The comb characteristics such as the number of lines and free-spectral range are defined at the AWG level. The polarization controller (PC) is used to align the laser polarization with the output of the modulator. The EO-comb is then amplified using an erbium-doped fiber amplifier (EDFA) to boost the comb’s optical power. To couple the light in and out of the photonic integrated circuit containing the MWL and the optical feedback cavity, we use a lensed fiber whose output is coupled to a fiber optic circulator (FOC) to avoid back reflections. The MWL output is then sent towards a high-resolution optical spectrum analyzer (APEX, AP2083, resolution down to 5 MHz or 40 fm), and a large bandwidth photodetector (Thorlabs, RXM42AF 42 GHz) coupled to an RF spectrum analyzer (Keysight, MXA-N9021B). We set the current applied to DBR1 and DBR2 of the MWL to IDBR1 = 0 mA and IDBR2 = 1 mA, respectively. We define the injection strength by measuring the optical power of the injected signal before the lensed fiber. The detuning Δ is defined as the frequency difference between the frequency of the middle line of the comb fm, and the free-running frequency of the mode under injection fs: Δ = fm − fs.

Numerical model and simulations

We use the multimode rate equation model introduced by Viktorov et al.38 derived from equations for solid-state lasers. Already normalized in time and extended to include the effect of optical feedback48, we have added an extra term in the field equation to account for modulated optical injection32. By using the frequency of the master laser as reference frequency, we can remove the explicit time dependence thus making them an autonomous set of delayed-differential equations. These equations read as:

$$\begin{array}{rcl}\frac{d{F}_{1}}{dt}&=&(1+i\alpha )({g}_{1}{N}_{1}-\frac{1-{g}_{1}}{2}){F}_{1}\\ &+&\kappa {e}^{-i{\theta }_{1}}{F}_{1}(t-\tau ){e}^{-i\Delta \tau }+{\kappa }_{{{{{{{{\rm{inj}}}}}}}}}m(t)-i\Delta {F}_{1},\end{array}$$
(1)
$$\frac{d{E}_{2}}{dt}=(1+i\alpha )({g}_{2}{N}_{2}-\frac{1-{g}_{2}}{2}){E}_{2}+\kappa {e}^{-i{\theta }_{2}}{E}_{2}(t-\tau ),$$
(2)
$$T\frac{d{N}_{1}}{dt}=P-{N}_{1}-(1+2{N}_{1})({g}_{1}| {E}_{1}{| }^{2}+{g}_{2}\beta | {E}_{2}{| }^{2}),$$
(3)

and

$$T\frac{d{N}_{2}}{dt}=P-{N}_{2}-(1+2{N}_{2})(\beta {g}_{1}| {E}_{1}{| }^{2}+{g}_{2}| {E}_{2}{| }^{2}).$$
(4)

With E1,2 being the normalized electrical field for modes 1 and 2 respectively, and N1,2, the normalized carrier population density. All variables and parameters are normalized and further details of the normalization can be found in the original work48. It is however worth noting that all time/frequency parameters are normalized by the photon lifetime τp. The linewidth enhancement factor is represented as α and the modal gains by g1,2. T is the the carrier lifetime (normalized by the photon lifetime) and P is the normalized pump parameter. The mode coupling mechanism is driven by a parameter β which models the cross-saturation. The optical feedback is introduced by the second terms of the field equations and is modeled by the feedback rate κ, the time-delay τ (normalized by the photon lifetime), and the feedback phase θ1,2. The latter depends on the wavelengths and is therefore different for modes 1 and 2. For the numerical results depicted in Fig. 5, optical feedback is not considered, i.e., κ = 0. The use of feedback as a control mechanism to switch between wavelengths is however demonstrated in the Supplementary Information, section 7. The optical injection is introduced in the last two terms of the first equation and modeled by the injection rate κinj, the modulation m(t) (with the time parameter t being normalized by the photon lifetime), and the detuning Δ, i.e. the normalized frequency difference, between the master laser and the injected mode. The first equation is written for F1(t) = E1(t)eiΔt, i.e., the electrical field E1 shifted in frequency by the detuning Δ to make the equation autonomous. We simulate the system using direct numerical integration with a Runge-Kutta 4th-order algorithm. In the simulation, the linewidth enhancement factor is set to α = 3 and T = 1000. The pump parameter P corresponds to a normalized laser injection current J so that P = (J − Jth)/2Jth, with Jth being the threshold current. Here, we use P = 0.5, corresponding to an injection current 2 times the laser threshold. To fix the power difference between the two modes of the MWL, we need to adjust both gain and cross-saturation parameters. Here, we fix g1 = 0.995 and consider two cases: 1) g2 = 0.827 with β1 = 0.88 and 2) g2 = 0.954 with β2 = 0.95. Both cases lead to a power difference of 40 dB between modes without injection or feedback. For numerical investigation as in the experiment, we inject a comb with five tones. To better compare it with the experimental observations, in Fig. 5 we have expressed both the FSR and the detuning values in Hz by assuming a photon lifetime of 3 ps. In particular, to simulate an FSR of about 1 GHz, we use a normalized FSR of 0.019 ( ≈ 2πfτp with f = 1 GHz and τp = 3 ps). To obtain the bandwidth and the total power of the combs we define a threshold for the power of the comb lines at 30 dB below the power of the strongest comb line. Only the comb lines that appear above the threshold are considered for the bandwidth and power calculation. To evaluate the repetition rate, we compute the average spacing between the comb lines that appear above the threshold.