Featured
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Room temperature magnetic materials from nanostructured diblock copolymers
Simple routes to self-assembling magnetic materials are elusive. Tew and colleagues produce copolymers containing cobalt complexes, which phase separate to give ferromagnetic properties at room temperature following heat treatment.
- Zoha M. AL-Badri
- , Raghavendra R. Maddikeri
- & Gregory N. Tew
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| Open AccessRole of mid-gap states in charge transport and photoconductivity in semiconductor nanocrystal films
Nanocrystals are used in light-emitting diodes and solar cells, but their charge transport in films is unclear. Here, the study of PbS nanocrystal films reveals the role of mid-gap states in their charge transport, suggesting different design needs for devices operated in dark (transistors) versus light (solar cells) conditions.
- Prashant Nagpal
- & Victor I. Klimov
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| Open AccessHigh pressure route to generate magnetic monopole dimers in spin ice
Spin ices are magnetic materials in which excitations equivalent to monopoles can occur. Using high-pressure techniques, Zhouet al. synthesize a new member of the spin ice family, Dy2Ge2O7, in which monopoles exist at higher densities, and can stabilize as dimers.
- H.D. Zhou
- , S.T. Bramwell
- & J.S. Gardner
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| Open AccessA germanate transparent conductive oxide
Transparent conducting oxides are wide bandgap conductors that have found a range of applications in optoelectronic devices. In this study, Hosono and colleagues fabricate the first transparent conducting oxide based on germanium.
- Hiroshi Mizoguchi
- , Toshio Kamiya
- & Hideo Hosono
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Chemical potential oscillations from nodal Fermi surface pocket in the underdoped high-temperature superconductor YBa2Cu3O6+x
It is unclear whether the Fermi surface in the normal state of underdoped cuprates is ambipolar or solely nodal. Here, measuring the second harmonic oscillations in underdoped YBa2Cu3O6+xreveals the origin as an oscillatory chemical potential, based on which a Fermi surface consisting of a nodal pocket is identified.
- Suchitra E. Sebastian
- , N. Harrison
- & G.G. Lonzarich
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Surfactant-enabled epitaxy through control of growth mode with chemical boundary conditions
Property coupling by heteroepitaxy is severely limited in material combinations with highly dissimilar bonding. This report presents a chemical boundary condition methodology to actively engineer two-dimensional film growth in such systems that otherwise collapse into island formation and rough morphologies.
- Elizabeth A. Paisley
- , Mark. D. Losego
- & Jon-Paul Maria
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Strong plasmonic enhancement of photovoltage in graphene
Photodetection is believed to be among the most promising potential applications for graphene. Here, by combining graphene with plasmonic nanostructures, the efficiency of graphene-based photodetectors is increased by up to two orders of magnitude.
- T.J. Echtermeyer
- , L. Britnell
- & K.S. Novoselov
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| Open AccessBethe-hole polarization analyser for the magnetic vector of light
Determining the direction of the magnetic field of light is important for optical applications. Here, scattering of light from a subwavelength aperture in a metal plane is shown to be governed by its magnetic vector, providing the magnetic field orientation independently of the electric field.
- H.W. Kihm
- , S.M. Koo
- & D.-S. Kim
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| Open AccessFermi-surface reconstruction by stripe order in cuprate superconductors
An electron pocket exists in the Fermi-surface of the high temperature superconductor YBa2Cu3Oy, but its origin is unknown. Here, YBa2Cu3Oy and La1.8−xEu0.2SrxCuO4 are both shown to exhibit Fermi-surface reconstruction, and in the latter, this is due to stripe order, suggesting that the same mechanism exists in YBa2Cu3Oy.
- F. Laliberté
- , J. Chang
- & Louis Taillefer
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Highly aligned carbon nanotube forests coated by superconducting NbC
Composites of carbon nanotubes and superconductors provide technologically important new, or improved, functionalities. Here, with a chemical solution approach, well-aligned carbon nanotube forests embedded in a superconducting NbC matrix are shown to effectively enhance the superconducting properties of NbC.
- G.F. Zou
- , H.M. Luo
- & Q.X. Jia
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| Open AccessFrom computational discovery to experimental characterization of a high hole mobility organic crystal
The development of new organic semiconductors with high mobility and air stability will facilitate their widespread application. In this Article,in silicoscreening of extended oligothiophenes leads to the synthesis of a high performance semiconductor.
- Anatoliy N. Sokolov
- , Sule Atahan-Evrenk
- & Alán Aspuru-Guzik
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Li(Zn,Mn)As as a new generation ferromagnet based on a I–II–V semiconductor
Ferromagnetic systems produced by the transition metal doping of semiconductors may be used as components of spintronic devices. Here, a new ferromagnet, Li1+y(Zn1-xMnx)As, is prepared in bulk quantities and shown to have a critical temperature approaching 50 K.
- Z. Deng
- , C.Q. Jin
- & Y.J. Uemura
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| Open AccessPhoton extrabunching in ultrabright twin beams measured by two-photon counting in a semiconductor
The second order correlation functiong(2) is used to test quantum correlation properties of light. Here, two-photon counting is used to measure g(2)and an extrabunching effect is demonstrated, providing evidence that two-photon counting is an appropriate method for measuring light beam photon correlations.
- F. Boitier
- , A. Godard
- & E. Rosencher
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Direct imaging of Joule heating dynamics and temperature profiling inside a carbon nanotube interconnect
The use of carbon nanotubes in nanoelectronics requires an understanding of their resistive, or Joule, heating at interconnects. Here, Joule heating dynamics are imaged in real time by following the evolution of resistive hot spots with a transmission electron microscope.
- Pedro M.F.J. Costa
- , Ujjal K. Gautam
- & Dmitri Golberg
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| Open AccessAdvantageous grain boundaries in iron pnictide superconductors
High critical temperature superconductors could be used to produce ideal electric power lines, but the misalignment of crystalline grain boundaries reduces current density. Here, pnictide superconductors are found to be more tolerant to misaligned grain boundaries than cuprates.
- Takayoshi Katase
- , Yoshihiro Ishimaru
- & Hideo Hosono
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| Open AccessMesoscale flux-closure domain formation in single-crystal BaTiO3
Flux-closure patterns are rarely observed in ferroelectric materials and almost exclusively form at the nanoscale. McQuaidet al. report mesoscopic dipole closure patterns formed in free-standing single-crystal lamellae of BaTiO3, thought to result from an unusual set of experimental conditions.
- R.G.P. McQuaid
- , L.J. McGilly
- & J.M. Gregg
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Encapsulation of single-molecule magnets in carbon nanotubes
Single-molecule magnets could be useful for the development of spintronic devices. Here single-molecule magnets are encapsulated in carbon nanotubes without affecting the properties of the guest molecules, which may be useful in the development of spintronic or high-density magnetic storage devices.
- Maria del Carmen Giménez-López
- , Fabrizio Moro
- & Andrei N. Khlobystov
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| Open AccessProximity of iron pnictide superconductors to a quantum tricritical point
In some iron-based materials, unconventional superconductivity can emerge near a quantum phase transition where long-range magnetic order vanishes. Giovannettiet al.show that the magnetic quantum phase transition in an iron pnictide superconductor is very close to the quantum tricritical point.
- Gianluca Giovannetti
- , Carmine Ortix
- & José Lorenzana
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| Open AccessGross violation of the Wiedemann–Franz law in a quasi-one-dimensional conductor
Interacting electrons in one dimension are predicted to have independent spin and charge excitations. Wakehamet al. show evidence of this behaviour in a bulk conductor by measuring a ratio of thermal to electrical conductivity orders of magnitude larger than in conventional three-dimensional metals.
- Nicholas Wakeham
- , Alimamy F. Bangura
- & Nigel E. Hussey
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| Open AccessFractional quantum Hall effect in the absence of Landau levels
The fractional quantum Hall effect occurs when electrons move in Landau levels. In this study, using a theoretical flat-band lattice model, the fractional quantum Hall effect is observed in the presence of repulsive interactions when the band is one third full and in the absence of Landau levels.
- D.N. Sheng
- , Zheng-Cheng Gu
- & L. Sheng
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Fermi surface dichotomy of the superconducting gap and pseudogap in underdoped pnictides
Iron pnictide compounds have recently been shown to have superconducting properties. Xuet al. show that the superconducting gap of underdoped pnictides scales linearly with the transition temperature, and that a pseudogap develops with underdoping.
- Y.-M. Xu
- , P. Richard
- & H. Ding
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| Open AccessOptical switching of nuclear spin–spin couplings in semiconductors
Two-qubit operation is an essential part of quantum computation, but implementation has been difficult. Gotoet al.introduce optically controllable internuclear coupling in semiconductors providing a simple way of switching inter-qubit couplings in semiconductor-based quantum computers.
- Atsushi Goto
- , Shinobu Ohki
- & Tadashi Shimizu
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Onset of a quantum phase transition with a trapped ion quantum simulator
A quantum simulator can follow the evolution of a prescribed model, whose behaviour may be difficult to determine. Here, the emergence of magnetism is simulated by implementing a quantum Ising model, providing a benchmark for simulations in larger systems.
- R. Islam
- , E.E. Edwards
- & C. Monroe
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Using disorder to detect locally ordered electron nematics via hysteresis
Interactions between charge, orbital and lattice degrees of freedom in correlated electron systems have resulted in predictions of new electronic phases of matter. Carlson and Dahmen propose two protocols for detecting disordered electron nematics in condensed matter systems using non-equilibrium methods.
- E.W. Carlson
- & K.A. Dahmen
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Imaging local electronic corrugations and doped regions in graphene
The unoccupied electronic levels of graphene are modified by corrugation, doping and presence of impurities. Here, the authors map discrete electronic domains within a single graphene sheet using scanning transmission X-ray microscopy and provide insight into the modification of unoccupied levels.
- Brian J. Schultz
- , Christopher J. Patridge
- & Sarbajit Banerjee
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| Open AccessSize limits the formation of liquid jets during bubble bursting
A bubble at an air–liquid interface can form a liquid jet upon bursting, spraying aerosol droplets into the air. Leeet al. show that jetting is analogous to pinching-off in liquid coalescence, which may be useful in applications that prevent jet formation and in the improved incorporation of aerosols in climate models.
- Ji San Lee
- , Byung Mook Weon
- & Wah-Keat Lee
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| Open AccessThe vectorial control of magnetization by light
Light–matter interactions can be used to manipulate magnetization in solids, but light-controlled magnetization vector motion has not been demonstrated. Here, two-dimensional magnetic oscillations in NiO are manipulated with optical pulses leading to vectorial control of magnetization by light.
- Natsuki Kanda
- , Takuya Higuchi
- & Makoto Kuwata-Gonokami
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Collective fluorescence enhancement in nanoparticle clusters
Single nanoparticles are known to emit light intermittently, or 'blink', but the mechanisms describing this phenomenon are not fully understood. This study demonstrates that, for small clusters of blinking nanoparticles, the number of particles within a cluster dramatically influences blinking time.
- Siying Wang
- , Claudia Querner
- & Marija Drndic
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| Open AccessPromotion of water-mediated carbon removal by nanostructured barium oxide/nickel interfaces in solid oxide fuel cells
Anodes composed of nickel/yttria-stabilized zirconia in solid oxide fuel cells are known to suffer from coking, which reduces their performance. Here, Yang and colleagues report a new barium oxide/nickel anode, which efficiently oxidizes fuel with minimum carbon buildup.
- Lei Yang
- , YongMan Choi
- & Meilin Liu
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| Open AccessRevealing the high-energy electronic excitations underlying the onset of high-temperature superconductivity in cuprates
Understanding how the high-energy physics of Mott-like excitations affects condensate formation is a key challenge in high-temperature superconductivity. Giannettiet al. clarify the relationship of many-body CuO2excitations and the onset of superconductivity using a new optical pump supercontinuum-probe technique.
- Claudio Giannetti
- , Federico Cilento
- & Fulvio Parmigiani
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| Open AccessColossal negative thermal expansion in BiNiO3 induced by intermetallic charge transfer
Negative thermal expansion—contraction upon heating—is an unusual process that may be exploited to produce materials with zero or other controlled thermal expansion values. Azumaet al. observe negative thermal expansion in BiNiO3which is a result of Bi/Ni charge-transfer transitions.
- Masaki Azuma
- , Wei-tin Chen
- & J. Paul Attfield
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| Open AccessTransition to a Bose–Einstein condensate and relaxation explosion of excitons at sub-Kelvin temperatures
Bose–Einstein condensation of excitons in thermal equilibrium is a predicted quantum statistical phenomenon that has been difficult to observe. Yoshiokaet al. cool trapped excitons to sub-Kelvin temperatures and show that condensation manifests itself as a relaxation explosion as has been observed for atomic hydrogen.
- Kosuke Yoshioka
- , Eunmi Chae
- & Makoto Kuwata-Gonokami
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| Open AccessActive microrheology and simultaneous visualization of sheared phospholipid monolayers
Two-dimensional fluid interfaces are ubiquitous, but studying their surface dynamic properties is difficult because of coupling between the film and bulk fluid. Choiet al.combine active microrheology with fluorescence microscopy to image fluid interfaces under applied stress.
- S.Q. Choi
- , S. Steltenkamp
- & T.M. Squires
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| Open AccessFractal fronts of diffusion in microgravity
Theory and simulations predict scale-invariant concentration fluctuations during diffusion in liquids, but on Earth, large-scale fluctuations are damped by gravity. Microgravity experiments by Vailatiet al. reveal the scale-invariant nature of diffusion, associated with fractal fronts and long-ranged correlations.
- Alberto Vailati
- , Roberto Cerbino
- & Marzio Giglio
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| Open AccessReversible temperature regulation of electrical and thermal conductivity using liquid–solid phase transitions
Temperature-controlled regulation of thermal conductivity is difficult to achieve because thermal properties do not change significantly through solid-state phase transitions. Here temperature control of thermal conductivities is demonstrated using liquid–solid phase transitions in a nanoparticle suspension.
- Ruiting Zheng
- , Jinwei Gao
- & Gang Chen
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Observation of atomic speckle and Hanbury Brown–Twiss correlations in guided matter waves
Speckle patterns are a manifestation of decoherence and can result from two-particle interference. Here, the authors image atomic speckle for guided matter waves and link this to atom bunching in the second-order correlation function, suggesting potential use in squeezed-atom interferometry applications.
- R.G. Dall
- , S.S. Hodgman
- & A.G. Truscott
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| Open AccessThe Meissner effect in a strongly underdoped cuprate above its critical temperature
In the pseudogap state of cuprates, although diamagnetic signals have been detected, a Meissner effect has never been observed. Morenzoni and colleagues probe the local diamagnetic response in the normal state of an underdoped layer showing that a 'barrier' layer exhibits a Meissner effect.
- Elvezio Morenzoni
- , Bastian M. Wojek
- & Ivan Božović
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Molecular dynamics of single-particle impacts predicts phase diagrams for large scale pattern formation
Energetic particle irradiation can lead to surface smoothing, pattern formation or degradation of the structural integrity of nuclear reactor components. Here, molecular dynamics simulations are used to study the mechanisms that determine the transitions between these disparate processes.
- Scott A. Norris
- , Juha Samela
- & Michael J. Aziz
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| Open AccessMagnetic vortex core reversal by excitation of spin waves
Micron and submicron-sized magnetic platelets in a vortex configuration may be useful in micromagnetics and spintronics applications. Kammereret al. show that a fast unidirectional vortex core reversal process occurs when azimuthal spin wave modes are excited at GHz frequency.
- Matthias Kammerer
- , Markus Weigand
- & Gisela Schuetz
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| Open AccessGapless spin liquid of an organic triangular compound evidenced by thermodynamic measurements
Frustrated magnetic systems can form an exotic quantum spin-liquid ground state, in which strongly correlated spins fluctuate in the spin lattices. Here, the low-temperature electronic state of a charge-transfer compound is found to form a gapless spin liquid.
- Satoshi Yamashita
- , Takashi Yamamoto
- & Reizo Kato
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Tip-enhanced photovoltaic effects in bismuth ferrite
Bismuth ferrite has photoelectric properties that make it an attractive alternative for use in photovoltaic devices. Here, using photoelectric atomic force microscopy, the authors show that photogenerated carriers can be collected by the tip and suggest that this can be used in photoelectric applications.
- Marin Alexe
- & Dietrich Hesse
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The lifetime of the deviations from bulk behaviour in polymers confined at the nanoscale
Monitoring the impact of annealing on nanometre-thick polymer layers provides new insight into the changes in the performance of macromolecular materials. Here, the authors present results showing a correlation between the deviations from bulk behaviour and the growth of an irreversibly adsorbed layer.
- Simone Napolitano
- & Michael Wübbenhorst
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Electrical injection and detection of spin accumulation in silicon at 500 K with magnetic metal/silicon dioxide contacts
Harnessing spin angular momentum could allow the development of electronic devices that are not limited by Moore's law. Here, electrical injection and detection of spin accumulation is achieved at temperatures that are practical for device operation.
- C.H. Li
- , O.M.J. van 't Erve
- & B.T. Jonker
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Quasi-two-dimensional Skyrmion lattices in a chiral nematic liquid crystal
Skyrmions are particle-like topological entities in a continuous field that have a role in various condensed matter systems. Here, numerical methods are used to show that a chiral nematic liquid crystal could be used as a model system to facilitate direct structural investigation of Skyrmions.
- Jun-ichi Fukuda
- & Slobodan Žumer
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Coherent electron–phonon coupling in tailored quantum systems
Graphene and InAs nanowires are both promising materials for coherent spin manipulation, but coupling between a quantum system and its environment leads to decoherence. Here, the contribution of electron–phonon coupling to decoherence in graphene and InAs nanowire is studied.
- P. Roulleau
- , S. Baer
- & T. Ihn
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Nanofriction in cold ion traps
Cold ion traps have not previously been used to study sliding friction between crystal lattices. Here, Benassiet al. use simulations to show that cold ion traps could be used for detailed investigation of atomic scale friction.
- A. Benassi
- , A. Vanossi
- & E. Tosatti
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Electrically controllable spontaneous magnetism in nanoscale mixed phase multiferroics
Complex oxide interfaces are important for electronic and spintronic applications. In this study, the authors show the emergence of spontaneous magnetism at one such interface between two phases of BiFeO3due to strain effects and piezoelectric coupling.
- Q. He
- , Y. -H. Chu
- & R. Ramesh
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| Open AccessPhonon-tunnelling dissipation in mechanical resonators
The performance of micromechanical and nanomechanical resonators is often hampered by mechanical damping. In this study, the authors demonstrate a numerical solver for the prediction of support-induced losses in these structures and verify experimentally the fidelity of this method.
- Garrett D. Cole
- , Ignacio Wilson-Rae
- & Markus Aspelmeyer
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| Open AccessFirst direct observation of the Van Hove singularity in the tunnelling spectra of cuprates
In two-dimensional lattices the electronic levels are unevenly spaced and the density of states exhibits a divergence known as the Van Hove singularity. In this study, the Van Hove singularity is observed for the first time in a cuprate using scanning tunnelling microscopy.
- A. Piriou
- , N. Jenkins
- & Ø. Fischer
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